LrgpV1, Main, Exploration, bibRecord, 000036

Driving Forces Controlling Host-Guest Recognition in Supercritical Carbon Dioxide Solvent.

Identifieur interne : 000036 ( Main/Exploration ); précédent : 000035; suivant : 000037

Driving Forces Controlling Host-Guest Recognition in Supercritical Carbon Dioxide Solvent.

Auteurs : Francesca Ingrosso [France] ; Muhannad Altarsha [France] ; Florence Dumarçay [France] ; Gwendal Kevern [France] ; Danielle Barth [France] ; Alain Marsura [France] ; Manuel F. Ruiz-L Pez [France]

Source :

Chemistry (Weinheim an der Bergstrasse, Germany) [ 1521-3765 ] ; 2016.

RBID : pubmed:26784687

Descripteurs français

KwdFr :
- Catalyse, Cyclodextrines bêta (), Dioxyde de carbone (), Solvants (), Structure moléculaire.
MESH :
- Catalyse, Cyclodextrines bêta, Dioxyde de carbone, Solvants, Structure moléculaire.

English descriptors

KwdEn :
- Carbon Dioxide (chemistry), Catalysis, Molecular Structure, Solvents (chemistry), beta-Cyclodextrins (chemistry).
MESH :
- chemical , chemistry : Carbon Dioxide, Solvents, beta-Cyclodextrins.
- Catalysis, Molecular Structure.

Abstract

The formation of supramolecular host-guest complexes is a very useful and widely employed tool in chemistry. However, supramolecular chemistry in non-conventional solvents such as supercritical carbon dioxide (scCO2 ), one of the most promising sustainable solvents, is still in its infancy. In this work, we explored a successful route to the development of green processes in supercritical CO2 by combining a theoretical approach with experiments. We were able to synthesize and characterize an inclusion complex between a polar aromatic molecule (benzoic acid) and peracetylated-β-cyclodextrin, which is soluble in the supercritical medium. This finding opens the way to wide, environmental friendly, applications of scCO2 in many areas of chemistry, including supramolecular synthesis, reactivity and catalysis, micro and nano-particle formation, molecular recognition, as well as enhanced extraction processes with increased selectivity.

DOI: 10.1002/chem.201503780
PubMed: 26784687

Affiliations:

Le document en format XML

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<front><div type="abstract" xml:lang="en">The formation of supramolecular host-guest complexes is a very useful and widely employed tool in chemistry. However, supramolecular chemistry in non-conventional solvents such as supercritical carbon dioxide (scCO2 ), one of the most promising sustainable solvents, is still in its infancy. In this work, we explored a successful route to the development of green processes in supercritical CO2 by combining a theoretical approach with experiments. We were able to synthesize and characterize an inclusion complex between a polar aromatic molecule (benzoic acid) and peracetylated-β-cyclodextrin, which is soluble in the supercritical medium. This finding opens the way to wide, environmental friendly, applications of scCO2 in many areas of chemistry, including supramolecular synthesis, reactivity and catalysis, micro and nano-particle formation, molecular recognition, as well as enhanced extraction processes with increased selectivity.</div>
</front>
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Driving Forces Controlling Host-Guest Recognition in Supercritical Carbon Dioxide Solvent.

Driving Forces Controlling Host-Guest Recognition in Supercritical Carbon Dioxide Solvent.

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English descriptors

Abstract

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